Preparation of Polymeric Hydrogel via Alternate Compression-Decompression

FU Wenbo; QIAO Pu; SHI Kaiyuan; SU Lei

doi:10.11858/gywlxb.20251042

Volume 39 Issue 9

Sep 2025

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Chinese Journal of High Pressure Physics > 2025 > 39(9): 093101.

FU Wenbo, QIAO Pu, SHI Kaiyuan, SU Lei. Preparation of Polymeric Hydrogel via Alternate Compression-Decompression[J]. Chinese Journal of High Pressure Physics, 2025, 39(9): 093101. doi: 10.11858/gywlxb.20251042

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FU Wenbo, QIAO Pu, SHI Kaiyuan, SU Lei. Preparation of Polymeric Hydrogel via Alternate Compression-Decompression[J]. Chinese Journal of High Pressure Physics, 2025, 39(9): 093101. doi: 10.11858/gywlxb.20251042

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Preparation of Polymeric Hydrogel via Alternate Compression-Decompression

doi: 10.11858/gywlxb.20251042

FU Wenbo^1
,,
QIAO Pu¹,
SHI Kaiyuan¹,
SU Lei^{1, 2,*
,
,}

1.
Center for High Pressure Science and Technology Advanced Research, Beijing 100193, China
2.
Shanghai Advanced Research in Physical Sciences, Shanghai 201203, China

Received Date: 04 Mar 2025
Rev Recd Date: 03 Apr 2025
Accepted Date: 20 May 2025

Available Online: 09 Apr 2025

Issue Publish Date: 05 Sep 2025

Abstract

Abstract

Based on the principles of gel preparation via freeze-thaw method and research progress in hydrogel synthesis, this study explores the effects of different pressure parameters systematically from the perspective of pressure regulation. Pressure magnitude, pressure compression and decompression rate, and number of cyclic loading were investigated during the gelation process of polymer solutions. By using the alternate compression-decompression (ACD) method, efficient and rapid synthesis of a series of hydrogels with excellent mechanical strength is enabled. These hydrogels have potential applications in diverse fields, including biomedicine, environmental protection, and electronic devices. As an innovative approach, the ACD method not only expands the preparation strategies for hydrogels significantly but also enhances the application potential of hydrogels in the field of soft matter science, providing new insights and directions for further development in this field.
- hydrogel,
- alternate compression-decompression method,
- pressure regulation

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References(24)

References

[1]	王薇, 关国平, 王璐. 生物医用水凝胶研究进展 [J]. 生物医学工程学进展, 2015, 36(4): 221–225. doi: 10.3969/j.issn.1674-1242.2015.04.008 WANG W, GUAN G P, WANG L. Research progress in biomedical hydrogels [J]. Progress in Biomedical Engineering, 2015, 36(4): 221–225. doi: 10.3969/j.issn.1674-1242.2015.04.008
[2]	谭燕, 刘曦, 袁芳. 魔芋葡甘聚糖的结构、性质及其在食品中的应用 [J]. 中国调味品, 2019, 44(2): 168–174, 178. doi: 10.3969/j.issn.1000-9973.2019.02.038 TAN Y, LIU X, YUAN F. Structure, properties of konjac glucomannan and its application in food industry [J]. China Condiment, 2019, 44(2): 168–174, 178. doi: 10.3969/j.issn.1000-9973.2019.02.038
[3]	CHEN X L, YANG T, CAI X L, et al. Eco-friendly hydrogel based on locust bean gum for water retaining in sandy soil [J]. International Journal of Biological Macromolecules, 2024, 275: 133490. doi: 10.1016/j.ijbiomac.2024.133490
[4]	ZHANG Y S, KHADEMHOSSEINI A. Advances in engineering hydrogels [J]. Science, 2017, 356(6337): eaaf3627. doi: 10.1126/science.aaf3627
[5]	饶涛, 何显儒. 高强度物理交联水凝胶综述 [J]. 塑料工业, 2022, 50(7): 6–11. doi: 10.3969/j.issn.1005-5770.2022.07.002 RAO T, HE X R. Review of high strength physical hydrogels [J]. China Plastics Industry, 2022, 50(7): 6–11. doi: 10.3969/j.issn.1005-5770.2022.07.002
[6]	LOZINSKY V I, PLIEVA F M, GALAEV I Y, et al. The potential of polymeric cryogels in bioseparation [J]. Bioseparation, 2001, 10: 163–188. doi: 10.1023/A:1016386902611
[7]	PEPPAS N A. Turbidimetric studies of aqueous poly (vinyl alcohol) solutions [J]. Die Makromolekulare Chemie, 1975, 176(11): 3433–3440. doi: 10.1002/macp.1975.021761125
[8]	LOZINSKY V I, DAMSHKALN L G, BROWN R, et al. Study of cryostructuring of polymer systems. XIX. on the nature of intermolecular links in the cryogels of locust bean gum [J]. Polymer International, 2000, 49(11): 1434–1443. doi: 10.1002/1097-0126(200011)49:11<1434::AID-PI525>3.0.CO;2-F
[9]	程慧茹, 张德坤. PVA-Silk复合水凝胶的摩擦磨损性能研究 [J]. 润滑与密封, 2010, 35(3): 14–18, 40. doi: 10.3969/j.issn.0254-0150.2010.03.004 CHENG H R, ZHANG D K. Research on the friction and wear properties of PVA-Silk composite hydrogel [J]. Lubrication Engineering, 2010, 35(3): 14–18, 40. doi: 10.3969/j.issn.0254-0150.2010.03.004
[10]	GRIGORYAN B, PAULSEN S J, CORBETT D C, et al. Multivascular networks and functional intravascular topologies within biocompatible hydrogels [J]. Science, 2019, 364(6439): 458–464. doi: 10.1126/science.aav9750
[11]	LEE J H, RIM Y S, MIN W K, et al. Biocompatible and biodegradable neuromorphic device based on hyaluronic acid for implantable bioelectronics [J]. Advanced Functional Materials, 2021, 31(50): 2107074. doi: 10.1002/adfm.202107074
[12]	SEDLAČÍK T, NONOYAMA T, GUO H L, et al. Preparation of tough double- and triple-network supermacroporous hydrogels through repeated cryogelation [J]. Chemistry of Materials, 2020, 32(19): 8576–8586. doi: 10.1021/acs.chemmater.0c02911
[13]	ADELNIA H, ENSANDOOST R, SHEBBRIN MOONSHI S, et al. Freeze/thawed polyvinyl alcohol hydrogels: present, past and future [J]. European Polymer Journal, 2022, 164: 110974. doi: 10.1016/j.eurpolymj.2021.110974
[14]	MIAO M S, SUN Y H, ZUREK E, et al. Chemistry under high pressure [J]. Nature Reviews Chemistry, 2020, 4(10): 508–527. doi: 10.1038/s41570-020-0213-0
[15]	QIAO P, SHI K Y, WANG Y L, et al. Ultrafast gelation of hyaluronan hydrogels via alternate compression-decompression [J]. Food Hydrocolloids, 2023, 141: 108732. doi: 10.1016/j.foodhyd.2023.108732
[16]	QIAO P, LI B, HE Y, et al. High-performance hydrogels via alternate compression-decompression [J]. The Journal of Physical Chemistry C, 2022, 126(51): 21825–21832. doi: 10.1021/acs.jpcc.2c06997
[17]	SU L, SHI K Y, ZHANG L, et al. Static and dynamic diamond anvil cell (s-dDAC): a bidirectional remote controlled device for static and dynamic compression/decompression [J]. Matter and Radiation at Extremes, 2022, 7(1): 018401. doi: 10.1063/5.0061583
[18]	LOZINSKY V I. Cryogels on the basis of natural and synthetic polymers: preparation, properties and application [J]. Russian Chemical Reviews, 2002, 71(6): 489–511. doi: 10.1070/RC2002v071n06ABEH000720
[19]	DE BRITO CARDOSO G, SOUZA I N, PEREIRA M M, et al. Poly(vinyl alcohol) as a novel constituent to form aqueous two-phase systems with acetonitrile: phase diagrams and partitioning experiments [J]. Chemical Engineering Research and Design, 2015, 94: 317–323. doi: 10.1016/j.cherd.2014.08.009
[20]	LIN S T, YUK H, ZHANG T, et al. Stretchable hydrogel electronics and devices [J]. Advanced Materials, 2016, 28(22): 4497–4505. doi: 10.1002/adma.201504152
[21]	BAKER M I, WALSH S P, SCHWARTZ Z, et al. A review of polyvinyl alcohol and its uses in cartilage and orthopedic applications [J]. Journal of Biomedical Materials Research. Part B, Applied Biomaterials, 2012, 100(5): 1451–1457. doi: 10.1002/jbm.b.32694
[22]	XU X, JHA A K, HARRINGTON D A, et al. Hyaluronic acid-based hydrogels: from a natural polysaccharide to complex networks [J]. Soft Matter, 2012, 8(12): 3280–3294. doi: 10.1039/C2SM06463D
[23]	BAKSH D, SONG L, TUAN R S. Adult mesenchymal stem cells: characterization, differentiation, and application in cell and gene therapy [J]. Journal of Cellular and Molecular Medicine, 2004, 8(3): 301–316. doi: 10.1111/j.1582-4934.2004.tb00320.x
[24]	ANSETH K S, METTERS A T, BRYANT S J, et al. In situ forming degradable networks and their application in tissue engineering and drug delivery [J]. Journal of Controlled Release, 2002, 78(1/2/3): 199–209. doi: 10.1016/S0168-3659(01)00500-4

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